Search results for "two-photon [exchange]"
showing 10 items of 56 documents
Single-shot generation and detection of a two-photon generalized binomial state in a cavity
2006
A "quasi-deterministic" scheme to generate a two-photon generalized binomial state in a single-mode high-Q cavity is proposed. We also suggest a single-shot scheme to measure the generated state based on a probe two-level atom that "reads" the cavity field. The possibility of implementing the schemes is discussed.
Two-photon exchange correction in elastic unpolarized electron-proton scattering at small momentum transfer
2015
We evaluate the two-photon exchange (TPE) correction to the unpolarized elastic electron-proton scattering at small momentum transfer $ Q^2 $. We account for the inelastic intermediate states approximating the double virtual Compton scattering by the unpolarized forward virtual Compton scattering. The unpolarized proton structure functions are used as input for the numerical evaluation of the inelastic contribution. Our calculation reproduces the leading terms in the $ Q^2 $ expansion of the TPE correction and goes beyond this approximation by keeping the full $ Q^2 $ dependence of the proton structure functions. In the range of small momentum transfer, our result is in good agreement with …
Two-photon spectroscopy of mercury and velocity-selective double resonances
2009
Two-photon laser spectroscopy of the $6\text{ }{^{1}S}_{0}\ensuremath{-}7\text{ }{^{1}S}_{0}$ transition in mercury has been performed using two copropagating continuous-wave laser beams. One laser beam is at 254 nm wavelength and can be tuned to the $6\text{ }{^{1}S}_{0}\ensuremath{-}6\text{ }{^{3}P}_{1}$ resonance. The other laser beam is at 408 nm. Two very different regimes can be distinguished, one far off resonance and one near resonance with the one-photon resonance. A resonance which is not Doppler broadened has been observed for low Rabi frequencies. This velocity-selective double resonance in a three-level ladder system is analogous to the dark resonance in three-level $\ensuremat…
Operation conditions and stability of a degenerate two-photon laser
1993
Abstract The presence of a far off-resonant intermediate level in a degenerate three-level two-photon laser model manifests through a steady pump-dependent and a dynamic frequency shift on the laser equations. The steady shift strongly affects the pump threshold necessary for emission, preventing it in certain cases. The dynamic shift makes the frequency pulling/pushing to be intensity-dependent and substantially modify the domains of existence and stability of the lasing solution permitting stable operation for large cavity losses in certain cases.
The role of nonlinear optical absorption in narrowband difference-frequency terahertz-wave generation
2010
We present a general analysis of the influence of nonlinear optical absorption on terahertz generation via optical difference frequency generation, when reaching for the quantum conversion efficiency limit. By casting the equations governing the process in a suitably normalized form, including either two-photon- or three-photon-absorption terms, we have been able to plot universal charts for phase matched optical-to-terahertz conversion for different values of the nonlinear absorption coefficients. We apply our analysis to some experiments reported to date, in order to understand to what extent multiphoton absorption could have played a role and also to predict the maximum achievable conver…
Quasi-spherical focal spot in two-photon scanning microscopy by three-ring apodization
2005
International audience; We present a beam-shaping technique for two-photon excitation (TPE) fluorescence microscopy. We show that by inserting a properly designed three-ring pupil filter in the illumination beam of the microscope, the effective optical sectioning capacity of such a system improves so that the point spread function gets a quasi-spherical shape. Such an improvement, which allows the acquisition of 3D images with isotropic quality, is obtained at the expense of only a small increase of the overall energy in the axial sidelobes. The performance of this technique is illustrated with a scanning TPE microscopy experiment in which the image of small beads is obtained. We demonstrat…
Light Sheet Fluorescence Microscopy (LSFM) for Two-Photon Excitation Imaging of Thick Samples.
2015
Over the last decades, fluorescence microscopy techniques have been developed in order to provide a deeper, faster and higher resolution imaging of three-dimensional biological samples. Within this framework, Light Sheet Fluorescence Microscopy (LSFM) became an increasingly useful and popular imaging technique able to answer several biological questions in the field of developmental biology [1]. Thanks to the spatial confinement of the excitation process within a thin sheet in the focal plane, it provides an intrinsic optical sectioning and a reduced phototoxicity. On the other side, Two-Photon Excitation (2PE), thanks to the use of IR wavelengths, has become an invaluable tool to improve i…
The Medium-Depending Fluorescence of Quadrupolar Donor-Acceptor-Donor Substituted Distyrylbenzenes with High Two-Photon Absorption Cross-Sections
2006
ABSTRACT1,4-Distyrylbenzenes with terminal dialkylamino groups and a central 2,5-disubstitution with electron-accepting groups were prepared via twofold Horner-olefination. These chromophores with a quadrupolar donor-acceptor-donor substitution and C2-symmetry absorb in the violet to green region of the visible spectrum exhibit large two-photon-absorption cross-sections when irrdiated in the NIR. Whereas a variation of the solvent polarity only slightly alters the absorption spectra, the fluorescence appears to be highly responsive. Besides a positive solvatochromism, the emission is very sensitive towards protonation. Quenching or appearance of new emitting species depends on the substitut…
Closed form for two-photon free–free transition matrix elements
2000
Abstract Two-photon free–free transitions happen in the multiphoton ionization with more than one excess photon and in bremsstralung. Up to now, the configuration space free–free transition amplitudes have not been written in closed form. We propose a modified Coulomb Green’s function (CGF) Sturmian expansion which allows one to obtain expressions for two-photon radial transition matrix elements in the closed form which are easy to continue analytically to calculate free–free transitions in H.
The electron beam induced short lived absorption in PLZT optical ceramics
2013
Abstract The short lived absorption induced by a pulsed electron beam in the led–lanthanum–zirconate–titanate (PLZT) optical ceramics was studied. The measured absorption spectrum covers 1.1–2.9 eV energy range and consists of several strongly overlapping peaks. The rise of the absorption is delayed with respect to the excitation pulse, due to charge carrier migration before trapping at centers responsible for the absorption. The formation rate of absorption centers and decay rate of absorption depend on the photon energy. The kinetics of short lived absorption varies over spectrum and can be approximated with a stretched exponent. The stretched exponent parameters indicate that the local d…